A General Copper-Box System for the Asymmetric Arylative Functionalization of Benzylic, Propargylic or Allenylic Radicals.

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成果类型：

期刊论文

作者：

Wang, Peng-Zi;Zhang, Zhihan;Jiang, Min;Chen, Jia-Rong;Xiao, Wen-Jing

作者机构：

[Xiao, Wen-Jing; Chen, Jia-Rong; Wang, Peng-Zi; Zhang, Zhihan] Engineering Research Center of Photoenergy Utilization for Pollution Control and Carbon Reduction, Ministry of Education

[Xiao, Wen-Jing; Chen, Jia-Rong; Wang, Peng-Zi; Zhang, Zhihan] College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei, 430079, China

[Jiang, Min] College of Materials, Chemistry and Chemical Engineering, Hangzhou Normal University, Hangzhou, 310036, China

[Xiao, Wen-Jing; Chen, Jia-Rong] Wuhan Institute of Photochemistry and Technology, 7 North Bingang Road, Wuhan, Hubei, 430083, China

语种：

英文

关键词：

arylation;asymmetric radical coupling;copper catalysis;photoredox catalysis

期刊：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

ISSN：

1433-7851

年：

2024

卷：

期：

页码：

e202411469

DOI：

10.1002/anie.202411469

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

Radical-involved arylative cross-coupling reactions have recently emerged as an attractive strategy to access valuable aryl-substituted motifs. However, there still exist several challenges such as limited scope of radical precursors/acceptors, and lack of general asymmetric catalytic systems, especially regarding the multicomponent variants. Herein, we reported a general copper-Box system for asymmetric three-component arylative radical cross-coupling of vinylarenes and 1,3-enynes, with oxime carbonates and aryl boronic acids. The reactions proceed under practical conditions in the absence or...

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A General Copper-Box System for the Asymmetric Arylative Functionalization of Benzylic, Propargylic or Allenylic Radicals.

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