Harmonizing Enzyme-like Cofactors to Boost Nanozyme Catalysis

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成果类型：

期刊论文

作者：

Wu, Yu;Zhong, Hong;Xu, Weiqing;Su, Rina;Qin, Ying;...

通讯作者：

Zhu, CZ;Guo, SJ

作者机构：

[Qin, Ying; Zhu, Chengzhou; Qiu, Yiwei; Gu, Wenling; Xu, Weiqing; Wu, Yu; Su, Rina; Zhu, CZ] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol &, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

[Zhong, Hong; Lin, Yuehe; Beckman, Scott P.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA.

[Zheng, Lirong] Chinese Acad Sci, Beijing Synchrotron Radiat Facil, Beijing 100049, Peoples R China.

[Hu, Liuyong] Wuhan Inst Technol, Hubei Engn Technol Res Ctr Optoelect & New Energy, Hubei Key Lab Plasma Chem & Adv Mat, Wuhan 430205, Peoples R China.

[Lv, Fan; Guo, SJ; Zhang, Shipeng; Guo, Shaojun] Peking Univ, Sch Mat Sci & Engn, Beijing 100871, Peoples R China.

通讯机构：

[Guo, SJ ] P

[Zhu, CZ ] C

Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol &, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

Peking Univ, Sch Mat Sci & Engn, Beijing 100871, Peoples R China.

语种：

英文

关键词：

Cofactors;Electron Transfer;Immunoassay;Metal–Organic Frameworks;Nanozymes

期刊：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

ISSN：

1433-7851

年：

2024

卷：

期：

页码：

e202319108-

DOI：

10.1002/anie.202319108

基金类别：

National Natural Science Foundation of China; Fundamental Research Funds for the Central Universities [CCNU22JC006]; Program of Introducing Talents of Discipline to Universities of China [B17019]; [22074049]; [22004042]

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

Engineering isolated metal sites resembling the primary coordination sphere of metallocofactors enables atomically dispersed materials as promising nanozymes. However, most existing nanozymes primarily focus on replicating specific metallocofactors while neglecting other supporting cofactors within active pockets, leading to reduced electron transfer (ET) efficiency and thus inferior catalytic performances. Herein, we report a metal–organic framework UiO-67 nanozyme with atomically dispersed iron sites, which involves multiple tailored enzyme-...

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Harmonizing Enzyme-like Cofactors to Boost Nanozyme Catalysis

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