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Renewable Energy Driven Electroreduction Nitrate to Ammonia and in-situ Ammonia Recovery via a Flow-Through Coupled Device

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成果类型:
期刊论文
作者:
Zhou, Bing;Zhan, Guangming;Yao, Yancai*;Zhang, Weixing;Zhao, Shengxi;...
通讯作者:
Zhang, LZ;Yao, Yancai
作者机构:
[Quan, Fengjiao; Zhang, Lizhi; Zhao, Shengxi; Fang, Chuyang; Huang, Yi; Jia, Falong; Zhang, LZ; Zhang, Weixing; Zhou, Bing] Cent China Normal Univ, Inst Environm & Appl Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China.
[Zhang, Lizhi; Yao, Yancai; Shi, Yanbiao; Zhang, LZ; Zhan, Guangming] Shanghai Jiao Tong Univ, Sch Environm Sci & Engn, Shanghai 200240, Peoples R China.
通讯机构:
[Yao, YC] S
[Zhang, LZ ] C
Cent China Normal Univ, Inst Environm & Appl Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China.
Shanghai Jiao Tong Univ, Sch Environm Sci & Engn, Shanghai 200240, Peoples R China.
语种:
英文
关键词:
Ammonia recovery;Cl-modified Cu electrode;Flow-through coupled device;Membrane-free electrolyzer;Nitrate electroreduction
期刊:
Water Research
ISSN:
0043-1354
年:
2023
卷:
242
页码:
120256
基金类别:
National Natural Science Foundation of China [U22A20402, 21936003, U21A20286, 22102100, 22206054]; National Key Research and Development Program of China [2021YFA1201701]; Key Program of Shenzhen Science and Technology Commission [JCYJ20220818095601002]; China Post-doctoral Science Foundation [2022M722080]; Natural Science Foundation of Shanghai [22ZR1431700]; Center for High Performance Computing at Shanghai Jiao Tong University
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
Green ammonia production from wastewater via electrochemical nitrate reduction contributes substantially to the realization of carbon neutrality. Nonetheless, the current electrochemical technology is largely limited by the lack of suitable device for efficient and continuous electroreduction nitrate into ammonia and in-situ ammonia recovery. Here, we report a flow-through coupled device composed of a compact electrocatalytic cell for efficient nitrate reduction and a unit to separate the produced ammonia without any pH adjustment and additiona...

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