Water-Soluble Metallo-Supramolecular Nanoreactors for Mediating Visible-Light-Promoted Cross-Dehydrogenative Coupling Reactions

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成果类型：

期刊论文

作者：

Han, Xin;Guo, Chenxing;Xu, Chen;Shi, Linlin;Liu, Binghui;...

通讯作者：

Wang, Heng(hengwang@szu.edu.cn);Hao, Xin-Qi(xqhao@zzu.edu.cn);Song, Mao-Ping(mpsong@zzu.edu.cn);Li, Xiaopeng(xiaopengli@szu.edu.cn)

作者机构：

[Hao, Xin-Qi; Zhu, Xinju; Song, Mao-Ping; Han, Xin; Liu, Binghui; Shi, Linlin] Zhengzhou Univ, Coll Chem, Green Catalysis Ctr, Zhengzhou 450001, Henan, Peoples R China.

[Lu, Shuai; Wang, Heng; Han, Xin; Guo, Chenxing; Li, Xiaopeng] Shenzhen Univ, Coll Chem & Environm Engn, Shenzhen 518055, Guangdong, Peoples R China.

[Guo, Chenxing] Shenzhen Univ, Sch Biomed Engn, Shenzhen 518060, Guangdong, Peoples R China.

[Xu, Chen] Jiangsu Univ Sci & Technol, Sch Environm & Chem Engn, Zhenjiang 212003, Jiangsu, Peoples R China.

[Zhang, Zhe; Bai, Qixia] Guangzhou Univ, Inst Environm Res Greater Bay Area, Key Lab Water Qual & Conservat Pearl River Delta, Minist Educ, Guangzhou 510006, Guangdong, Peoples R China.

通讯机构：

[Heng Wang; Xiaopeng Li] C

[Xin-Qi Hao; Mao-Ping Song] G

Green Catalysis Center, College of Chemistry, Zhengzhou University, Zhengzhou, Henan 450001, China<&wdkj&>College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen, Guangdong 518055, China

语种：

英文

关键词：

self-assembly;water-soluble metallo-supramolecular cages;nanoreactors;photochemical cross-coupling reactions;supramolecular catalysis

期刊：

ACS Nano

ISSN：

1936-0851

年：

2023

卷：

期：

页码：

3723–3736

DOI：

10.1021/acsnano.2c10856

基金类别：

National Natural Science Foundation of China [22125106, 21672192, 21803059, 22001176, U2004191, U1904212]; Devel- opmental Fund for Science and Technology of Shenzhen government [RCJC20200714114556036]; Tencent Funders Alumni Foundation

机构署名：

本校为其他机构

院系归属：

化学学院

摘要：

Water-soluble metallo-supramolecular cages with well-defined nanosized cavities have a wide range of functions and applications. Herein, we design and synthesize two series of metallo-supramolecular octahedral cages based on the self-assembly of two congeneric truxene-derived tripyridyl ligands modified with two polyethylene glycol (PEG) chains, i.e., monodispersed tetraethylene glycol (TEG) and polydispersed PEG-1000, with four divalent transition metals (i.e., Pd, Cu, Ni, and Zn). The resulting monodispersed cages C1-C4 are fully characterize...

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Water-Soluble Metallo-Supramolecular Nanoreactors for Mediating Visible-Light-Promoted Cross-Dehydrogenative Coupling Reactions

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